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• 1. [Article] ZnO Nanoneedle/H2O Solid-Liquid Heterojunction-Based Self-Powered Ultraviolet Detector

  ZnO nanoneedle arrays were grown vertically on a fluorine-doped tin oxide-coated glass by hydrothermal method at a relatively low temperature. A self-powered photoelectrochemical cell-type UV detector ...

  Citation × Citation Citation Abstract Copy Title: ZnO Nanoneedle/H2O Solid-Liquid Heterojunction-Based Self-Powered Ultraviolet Detector Author: Li, Qinghao, Wei, Lin, Xie, Yanru, Zhang, Kai, Liu, Lei, Zhu, Dapeng, Jiao, Jun, Chen, Yanxue, Yan, Shishen, Liu, Guolei, Mei, Liangmo Year: 2013 ZnO nanoneedle arrays were grown vertically on a fluorine-doped tin oxide-coated glass by hydrothermal method at a relatively low temperature. A self-powered photoelectrochemical cell-type UV detector was fabricated using the ZnO nanoneedles as the active photoanode and H2O as the electrolyte. This solid-liquid heterojunction offers an enlarged ZnO/water contact area and a direct pathway for electron transport simultaneously. By connecting this UV photodetector to an ammeter, the intensity of UV light can be quantified using the output short-circuit photocurrent without a power source. High photosensitivity, excellent spectral selectivity, and fast photoresponse at zero bias are observed in this UV detector. The self-powered behavior can be well explained by the formation of a space charge layer near the interface of the solid-liquid heterojunction, which results in a built-in potential and makes the solid-liquid heterojunction work in photovoltaic mode. Title: ZnO Nanoneedle/H2O Solid-Liquid Heterojunction-Based Self-Powered Ultraviolet Detector Author: Li, Qinghao, Wei, Lin, Xie, Yanru, Zhang, Kai, Liu, Lei, Zhu, Dapeng, Jiao, Jun, Chen, Yanxue, Yan, Shishen, Liu, Guolei, Mei, Liangmo Year: 2013 ZnO nanoneedle arrays were grown vertically on a fluorine-doped tin oxide-coated glass by hydrothermal method at a relatively low temperature. A self-powered photoelectrochemical cell-type UV detector was fabricated using the ZnO nanoneedles as the active photoanode and H2O as the electrolyte. This solid-liquid heterojunction offers an enlarged ZnO/water contact area and a direct pathway for electron transport simultaneously. By connecting this UV photodetector to an ammeter, the intensity of UV light can be quantified using the output short-circuit photocurrent without a power source. High photosensitivity, excellent spectral selectivity, and fast photoresponse at zero bias are observed in this UV detector. The self-powered behavior can be well explained by the formation of a space charge layer near the interface of the solid-liquid heterojunction, which results in a built-in potential and makes the solid-liquid heterojunction work in photovoltaic mode. Close

• 2. [Article] CdS Quantum Dot-Sensitized Solar Cells Based on Nano-Branched TiO2 Arrays

  Nano-branched rutile TiO2 nanorod arrays were grown on F:SnO2 conductive glass (FTO) by a facile, two-step wet chemical synthesis process at low temperature. The length of the nanobranches was tailored ...

  Citation × Citation Citation Abstract Copy Title: CdS Quantum Dot-Sensitized Solar Cells Based on Nano-Branched TiO2 Arrays Author: Liu, Chang, Li, Yitan, Wei, Lin, Wu, Cuncun, Chen, Yanxue, Mei, Liangmo, Jiao, Jun Year: 2014 Nano-branched rutile TiO2 nanorod arrays were grown on F:SnO2 conductive glass (FTO) by a facile, two-step wet chemical synthesis process at low temperature. The length of the nanobranches was tailored by controlling the growth time, after which CdS quantum dots were deposited on the nano-branched TiO2 arrays using the successive ionic layer adsorption and reaction method to make a photoanode for quantum dot-sensitized solar cells (QDSCs). The photovoltaic properties of the CdS-sensitized nano-branched TiO2 solar cells were studied systematically. A short-circuit current intensity of approximately 7 mA/cm2 and a light-to-electricity conversion efficiency of 0.95% were recorded for cells based on optimized nano-branched TiO2 arrays, indicating an increase of 138% compared to those based on unbranched TiO2 nanorod arrays. The improved performance is attributed to a markedly enlarged surface area provided by the nanobranches and better electron conductivity in the one-dimensional, well-aligned TiO2 nanorod trunks Title: CdS Quantum Dot-Sensitized Solar Cells Based on Nano-Branched TiO2 Arrays Author: Liu, Chang, Li, Yitan, Wei, Lin, Wu, Cuncun, Chen, Yanxue, Mei, Liangmo, Jiao, Jun Year: 2014 Nano-branched rutile TiO2 nanorod arrays were grown on F:SnO2 conductive glass (FTO) by a facile, two-step wet chemical synthesis process at low temperature. The length of the nanobranches was tailored by controlling the growth time, after which CdS quantum dots were deposited on the nano-branched TiO2 arrays using the successive ionic layer adsorption and reaction method to make a photoanode for quantum dot-sensitized solar cells (QDSCs). The photovoltaic properties of the CdS-sensitized nano-branched TiO2 solar cells were studied systematically. A short-circuit current intensity of approximately 7 mA/cm2 and a light-to-electricity conversion efficiency of 0.95% were recorded for cells based on optimized nano-branched TiO2 arrays, indicating an increase of 138% compared to those based on unbranched TiO2 nanorod arrays. The improved performance is attributed to a markedly enlarged surface area provided by the nanobranches and better electron conductivity in the one-dimensional, well-aligned TiO2 nanorod trunks Close